Driving Adsorbate Evolution via Oxygenated Surface Species Modulation for Ammonia Electrooxidation

  • Kim, Jeong Won
  • Hang, Yu Cheng
  • Park, Hyun Do
  • Cheng, Lin lin
  • Gong, Mingming
  • ... Shin, Hee Jong
  • 외 4명
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초록

Machine unlearning aims to selectively remove specific knowledge from a trained model. Existing approaches, such as Task Arithmetic, finetune the model on the forget set to create a task vector (i.e., a direction in weight space) for subtraction from the original model’s weight. However, their effectiveness is highly sensitive to hyperparameter selection, requiring extensive validation to identify the optimal vector from many fine-tuned candidates. In this paper, we propose a novel method that utilizes all fine-tuned models trained with varying hyperparameters instead of a single selection. Specifically, we aggregate the computed task vectors by retaining only the elements with consistent shared signs. The merged task vector is then negated to induce unlearning on the original model. Evaluations on zero-shot and standard image recognition tasks across twelve datasets and four backbone architectures show that our approach outperforms state-ofthe-art methods while requiring similar or fewer computational resources. Code is available at https://github.com/naver-ai/negmerge.

키워드

AlloyAmmoniaHydroperoxideIn situ FT-IRSurface activationWastewaterHYDROGENREDUCTIONEFFICIENTELECTROCATALYSTSELECTROLYSISOXIDATIONCATALYSTSIR
제목
Driving Adsorbate Evolution via Oxygenated Surface Species Modulation for Ammonia Electrooxidation
저자
Kim, Jeong WonHang, Yu ChengPark, Hyun DoCheng, Lin linGong, MingmingShah, Aamir HassanShin, Hee JongYe, CaichaoKim, Dong HaBu, Yunfei
DOI
10.1002/anie.202523481
발행일
2026-01
유형
Article
저널명
Angewandte Chemie - International Edition
65
4