Electrocatalytic Conversion of Carbon Dioxide and Nitrate Ions to Urea by a Titania-Nafion Composite Electrode

  • Saravanakumar, Duraisamy
  • Song, Jieun
  • Lee, Sunhye
  • Hur, Nam Hwi
  • Shin, Woonsup
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131
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133

초록

CO2 and nitrate ions were successfully converted to urea by a TiO2-Nafion nanocomposite electrode under ambient conditions. The composite electrode was constructed by dropcasting the mixture of P25 titania and Nafion solution on an indium-doped tin oxide (ITO) electrode. When the electrode was electrolyzed in CO2-saturated 0.1m KNO3 (pH4.5) solution at -0.98V versus Ag/AgCl, urea was formed with a Faradaic efficiency of 40%. The other reduced products obtained were NH3, CO, and H-2.

키워드

carbon dioxide conversionelectrocatalystindium-doped tin oxidetitanium oxideureaGAS-DIFFUSION ELECTRODESELECTROCHEMICAL SYNTHESISPHOTOCATALYTIC REDUCTIONNITRITE IONSMETAL-CATALYSTSCO2 CONVERSIONSIO2 MATRICESFUEL-CELLSTIO2WATER
제목
Electrocatalytic Conversion of Carbon Dioxide and Nitrate Ions to Urea by a Titania-Nafion Composite Electrode
저자
Saravanakumar, DuraisamySong, JieunLee, SunhyeHur, Nam HwiShin, Woonsup
DOI
10.1002/cssc.201701448
발행일
2017-10-23
유형
Article
저널명
ChemSusChem
10
20
페이지
3999 ~ 4003