Chitosan-Cross-linked Osmium Polymer Composites as an Efficient Platform for Electrochemical Biosensors

  • Jirimali, Harishchandra Digambar
  • Nagarale, Rajaram Krishna
  • Lee, Jong Myung
  • Saravanakumar, Durai
  • Shin, Woonsup
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초록

A new family of chitosan-cross-linked osmium polymer composites was prepared and its electrochemical properties were examined. The composites were prepared by quaternization of the poly(4-vinylpyridine) osmium bipyridyl polymer (PVP-Os) which was then cross-linked with chitosan, yielding PVP-Os/chitosan. Films made of the composites showed improved mass and electron transport owing to the porous and hydrophilic structure which is derived from the cross-links between the Os polymer and chitosan. The rate for glucose oxidation was enhanced four times when glucose oxidase (GOx) was immobilized on PVP-Os/chitosan compared immobilization on PVP-Os.

키워드

chitosan compositeselectron transferglucose sensorspolymersporous filmsHYDROGEN-PEROXIDE BIOSENSORGLUCOSE BIOSENSORREDOXELECTRODEENZYMESNANOCOMPOSITENANOPARTICLESCATALYSISLINKINGLACCASE
제목
Chitosan-Cross-linked Osmium Polymer Composites as an Efficient Platform for Electrochemical Biosensors
저자
Jirimali, Harishchandra DigambarNagarale, Rajaram KrishnaLee, Jong MyungSaravanakumar, DuraiShin, Woonsup
DOI
10.1002/cphc.201300169
발행일
2013-07-22
유형
Article
저널명
ChemPhysChem
14
10
페이지
2232 ~ 2236