K4GeP4Se12: a case for phase-change nonlinear optical chalcogenide

  • Jang, J. I.; 
  • Park, S.; 
  • Harrison, C. M.; 
  • Clark, D. J.; 
  • Morris, C. D.; 
  • 외 2명
Citations

WEB OF SCIENCE

23
Citations

SCOPUS

25

초록

We report on broadband nonlinear optical (NLO) responses from a phase-change chalcogenide compound K4GeP4Se12. Its glassy phase exhibits unusual second-harmonic generation (SHG) due to the preservation of local crystallographic order. The SHG efficiency of the glassy form can be boosted by more than 2 orders of magnitude by simple heat treatment. Strong SHG and third-harmonic generation from both glassy and crystalline compounds were characterized over a wide wavelength range of 1.2-4.0 mu m. Our results imply that K4GeP4Se12 can be utilized for various NLO applications in the mid-infrared spectrum. (C) 2013 Optical Society of America

키워드

2ND-HARMONIC GENERATION; FREQUENCY-GENERATION; GLASS-FIBERS; RB; RADIATION
제목
K4GeP4Se12: a case for phase-change nonlinear optical chalcogenide
저자
Jang, J. I.; Park, S.; Harrison, C. M.; Clark, D. J.; Morris, C. D.; Chung, I.; Kanatzidis, M. G.
DOI
10.1364/OL.38.001316
발행일
2013-04-15
유형
Article
저널명
Optics Letters
권
38
호
8
페이지
1316 ~ 1318